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《Showcasing research from Professor Wei Wang’s laboratory,School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, China.展示王瑋教授實(shí)驗(yàn)室地研究成果, 南京化學(xué)化工學(xué)院 中國南京大學(xué).pdf》由會(huì)員上傳分享,免費(fèi)在線閱讀,更多相關(guān)內(nèi)容在教育資源-天天文庫。
1、ShowcasingresearchfromProfessorWeiWang’slaboratory,Asfeaturedin:SchoolofChemistryandChemicalEngineering,NanjingUniversity,Nanjing,China.MonitoringthedynamicphotocatalyticactivityofsingleCdSnanoparticlesbylightingupH2nanobubbleswith?uorescentdyesStudyingthesemiconducto
2、rphotocatalysisatsinglenanoparticlelevelisdesiredforunderstandingthemicroscopicreactionkineticsandmechanismwithimplicationsfordesigningbettercatalysts.Inthepresenceofhydrophobic?uorescentdyes,individualH2nanobubblesgeneratedduringthephotocatalysisofsingleCdSnanopartic
3、leswerevisualizedunderconventional?uorescentmicroscopybecauseitrecruitedandaccumulated?uorescentdyesattheliquid-gasinterface.Inthismanner,thephotocatalyticSeeWeiWangetal.,activityofsingleCdSnanoparticlecanbemonitoredandChem.Sci.,2018,9,1448.quanti?ed,whichwasfoundtody
4、namically?uctuateamonghighactivity,lowactivityandinactivestates.rsc.li/chemical-scienceRegisteredcharitynumber:207890ChemicalScienceViewArticleOnlineEDGEARTICLEViewJournal
5、ViewIssueMonitoringthedynamicphotocatalyticactivityofsingleCdSnanoparticlesbylightingupH2Citethi
6、s:Chem.Sci.,2018,9,1448nanobubbleswith?uorescentdyes?HuaSu,YiminFang,FangyuanChenandWeiWang*Thecapabilityofsemiconductornanomaterialstoconvertsolarenergytochemicalenergyhasledtomanypromisingapplications,forinstance,photocatalyzedH2generation.Studyingthisimportantphoto
7、catalyticreactionatthesinglenanocatalystlevelprovidesagreatopportunitytounderstandthemicroscopicreactionkineticsandmechanismbyovercomingthechemicalandstructuralheterogeneityamongindividuals.Herewereporta?uorescence(FL)labelingstrategytovisualizeindividualH2nanobubbles
8、thataregeneratedatsingleCdSnanoparticlesduringphotocatalysis.Inoperandoimagingofnanobubblegrowthkineticsallowsfordeterminationofthephotocatalyticactivityofsinglenanocatalysts,whichwasfoundtorandomlyalternateamonghighactivity,lowactivityandinactiveCreativeCommonsAttrib
9、ution-NonCommercial3.0UnportedLicence.states.InadditiontoH2nanobubbles,thepresentlabelingstrategyisalsosuitableforothertypes